Sunday, 25 December 2016

Non-Linear Modes in Lithium Niobate Ferroelectrics with niobium antisite defects

Ferroelectric belongs to an important class of materials showing very interesting non-linear optical properties that have a variety of application in photonic devices In a discrete Hamiltonian, if we consider the space and time dependence of polarization vectors with an interaction term between two polarization domains, it gives rise to a nonlinear Klein-Gordon (K-G) equation that has been shown in some systems [Phys. Rev. B 86, 184101 (2012), and Phys. Rev.-B 81, 064104 (2010)]. This equation as a governing equation enables multiple time-scale analysis (MTSA) to be performed on a real ferroelectric material that reveals new type of information on both linear (known as soft modes) and the nonlinear parts of frequencies and amplitudes of oscillations. MTSA was described in a K-G system based on staggered polarization where more emphasis was given to reveal the presence of intrinsic localized modes (ILM). Here, detailed results for the first three linear modes and their frequencies as a function of a wide range of niobium antisite defects or, impurities in lithium niobate ferroelectric are presented. It is found that when an external excitation (i.e. the input) is only harmonic in nature, it could not be ascertained whether the even modes of the solitonic waves (i.e. the output) will have phase-locking with this type of harmonic external force.

The paper is organized as follows: In Section II, a brief description of the MTSA technique is given, in both linear and nonlinear forms, and at the end of this section three cases are presented for electric field and damping. In Section III, the results and discussion are given for linear modes and frequencies that are shown to depend on impurity content of lithium niobate as well as on upper limit of domain wall width. In Section III, the nonlinear modes, their frequencies and amplitudes are also shown. In Section IV, the conclusions are given.
A Bhattacharya, K Choudhary, S Das, L Vu-Quoc, and A K Bandyopadhyay - arXiv preprint arXiv: …, 2016

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