Friday, 12 October 2012

Discrete Energy Level of Bright Soliton in Lithium Niobate Ferroelectrics


Abstract:                                                                           

In the framework of a simple model of one dimensional array of ferroelectric slab of domains, the polarization with time and space is explained by Klein-Gordon equation. A perturbation of K-G equation makes it possible to use this continuum model through progressive wave nonlinear Schrodinger equation (NLSE). The latter gives rise to bright soliton that moves with certain velocity. The bright soliton controls itself so that both bright and dark solitons appear at the same time with discrete energy levels that is estimated from a hypergeometric function, but dark soliton is not visible as it is part of the complex solution that indicates absorption of energy, i.e. the presence of an energy-gap. The pulse width for switching of ferroelectrics can be estimated from the analysis of NLSE that matches with that calculated from this model.

Keyword: Bright Soliton, Discrete Energy Level, Hypergeometric Function, Ferroelectrics.

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In this work, the validity of NLSE breaks down near collapse where the assumption of small amplitude and large scale of modulation no longer holds. The effects of perturbations that can modify or even arrest the collapse are also considered. These include dissipation, normal dispersion and saturated nonlinearity. Both bright and dark solitons are the solutions of NLSE under the conditions: group velocity is higher or lower than coupling. The bright soliton moves with a velocity of 37.73 m/see and dark soliton moves with a velocity of 0.43 m/see for coupling=10. The soliton has self-energy or amplitude and this has important role in controlling bright soliton so that bright soliton has discrete energy levels. When wave packet passes through lithium niobate ferroelectrics, the dispersion will take place near the domain wall and in the absence of dispersion, the soliton will appear near the domain wall. When bright soliton passes through self-energy barrier, it splits into real and imaginary parts, i.e. bright and dark solitons respectively with discrete energy levels. It also implies a band-gap for the complex solution.
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Phys. Rev. B, Vol. 86, 184101, (2012)   

Friday, 17 August 2012

Fano resonance due to Discrete Breather in Nonlinear Klein-Gordon Lattice in Metamaterials


Abstract: The richer variety of Klein-Gordon basis is already established for discrete breathers in metamatetrials. Based on this attempt, we show various anomalous Fano-resonance behaviors that have been experimentally observed, but cannot be explained by nonlinear Schrodinger model. Certain material parameters of K-G lattice in metamaterials are related for the first time with characteristics of Fano-resonance, which can be utilized for beam filtering and for high-resolution biological sensing technology. Although relations with coupling and other parameters exist, the most remarkable relation is observed with linear permittivity that could control the wave transmission characteristics in metamaterials for applications in optical engineering. 
Keywords: Fano Resonance, Discrete Breathers, Klein-Gordon Lattice, Metamaterials.
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The novelty of this work is to deal with the physics of Fano resonance in case of discrete breathers in metamaterials in a Klein-Gordon lattice in terms of various material parameters, which may not be explained by nonlinear Schrodinger equation (NLSE). Discrete breathers could affect the energy transport by scattering phonons similar to impurity in mesoscopic transport system giving rise to open and closed channels. The closed channel is considered to be generated in the localized regime by the discrete breathers where the interaction with the THz radiation could be intense and hence this also gives rise to the opportunity for beam-filtering. In literature, there is almost no work on metamaterials related to the application of Klein-Gordon equation for Fano resonance. Hence, certain material parameters of K-G lattice in such materials are related for the “first time” with characteristics of Fano-resonance. So, our main focus is to show how the material parameters of  K-G lattice influence the performance of metamaterials in terms of bio-sensitivity, spectral selectivity, etc.
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J. Optical Soc. of America – B, Vol. 29 [9], 2414-19 (2012).

Thursday, 14 June 2012

Role of Coupling of Discrete Breathers in SRR based Metamaterials

Abstract:
The presence of classical discrete breathers and then a two-phonon bound state (TPBS) or quantum breather (QB) state through detailed quantum calculations have already been shown in nonlinear photonic materials, such as ferroelectrics. The latter was done in a periodic boundary condition in terms of variations of TPBS parameters against impurity that is related to nonlinearity. Metamaterials are also nonlinear optical materials for applications as split-ring-resonator (SRR) in the antenna arrays. By using a Klein-Gordon approach, first multi-solitons and classical breathers are shown. For QBs, by using a periodic boundary condition, the variation of the TPBS parameters with coupling within the SRR elements is observed. Finally, in a non-periodic boundary condition approach, the temporal evolution of number of quanta is shown eventually to derive the critical time of redistribution of quanta that is proportional to QB’s lifetime in femtosecond, which also shows variation with coupling in the SRR system.

Keywords: Metamaterials, Discrete Breathers, Klein-Gordon Lattice, Quantum Breathers
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Our main focus is directed towards temporal evolution of such quantum breathers in a non-periodic boundary condition approach with an eye on THz applications, as these engineered materials show a large magnetic response at THz frequency. This has also application in quantum computation, as the coherent quantum dynamics of ‘qubits’ determines the THZ optical properties in the system.
(Physica Scripta, Vol. 86 (2012) 015601)

Monday, 11 June 2012

Klein-Gordon Equation Approach to Non-linear Split Ring Resonator Based Metamaterials: 1D Systems

Abstract:
The electrodynamics of a one-dimensional split-ring resonator (SRR) based nonlinear metamaterial is studied.  The metamaterial is a one-dimensional periodic array of weakly coupled SRRs, with each SRR represented by a nonlinear resistor-inductor-capacitor (RLC) equivalent resonator circuit.  Nonlinearity is introduced into the system by the addition of Kerr-type dielectric medium within the SRRs or by the introduction into the system of certain other nonlinear elements (e.g., diodes). In the continuum limit of the system, variations of the charge stored within the capacitive slits in the SRRs in both time and space are shown to be described along the array by a nonlinear Klein-Gordon equation. Analytical solutions of the nonlinear K-G equation for both dark and bright solutions, breather, and pulse soliton solutions are obtained and studied.  A discussion is given of the relationship between the K-G solutions and solutions of the nonlinear Schrodinger equation (NLSE) approximation to the NLKG equation. A comparison is made of the K-G solutions with intrinsic localized mode (discrete breather) solutions of the discrete system and their continuum limits.  An additional continuum limit differential equation for the breather mode is obtained which is not bound by a weak coupling assumption, and its relation to the K-G equation is studied. Analytic forms are given for the effect of dissipation in the system on the various dark and bright envelope, breather and pulse solitons. Discussions are given of the effects of further than first neighbor couplings in the SRR system.
Keywords: Metamaterials, NLKG equation, Dark & Bright Envelop, Breather and Pulse Solitons.
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For the first time, metamaterials are described by NLKG equation that is found to be a richer variety than NLSE. A detailed comparison shows that both NLKG and NLSE show dark and bright envelop solitons and discrete breathers, but NLKG in addition shows breather pulses, whereas NLSE does not show such pulses. This should trigger further studies on the subject of metamaterials for antenna and other applications in the THz regime.
(Phys. Rev. B, Vol. 84 (2011) 155429)

Quantum Breathers in Klein-Gordon Lattice: Non-Periodic Boundary Condition Approach

Abstract:
The presence of classical breathers and two-phonon bound state (TPBS) or quantum breather (QB) state through detailed quantum calculations have already been shown in technologically important ferroelectric materials, such as lithium niobate with antisite niobium charge defects concerning  pinning transition, its control and application. The latter was done in a periodic boundary condition with Bloch function in terms of significant variations of TPBS parameters against impurity, which is related to nonlinearity. In further extension of this work, in a non-periodic boundary condition and number conserving approach, apart from various techniques available, only the temporal evolution of the number of quanta (i.e. phonons) in more sites is detailed in this present investigation for a generalized Klein-Gordon system with applications in ferroelectrics, metamaterials, and DNA. The critical time of redistribution of quanta that is proportional to QB’s lifetime in these materials show different types of behaviour in the femtosecond range, which give rise to the possibilities for making various devices.
Keywords: Quantum Breathers, Klein-Gordon Lattice, Non-Periodic Boundary Condition, Temporal Evolution of Quanta.
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In a non-periodic boundary condition, making our generalized Hamiltonian in Klein-Gordon lattice time dependent, the temporal evolution of quanta shows criticality that is proportional to QB’s lifetime in femtoseconds. The responses in the femtosecond regime of ferroelectrics, metamaterials and DNA are studied together to get an overview of different materials. This effort paves the way for various applications in the THz frequency as well as in quantum computation.
(J. Appl. Phys., Vol. 110 (2011) 124106)

Sunday, 10 June 2012

Quantum Pinning-transition due to Charge Defects in Ferroelectrics

Abstract:
We investigate pinning of domain walls in ferroelectrics on the basis of two phonon bound state (TPBS) or discrete breather state due to impurity energy levels above the phonon continua in ferroelectrics such as LiNbO3 to show pinning transition, which indicates the point of easiest switching. We predict with the help of our quantum calculations that every ferroelectric material has such a critical point of easy switching. Here we describe the quantum origin of pinning through the findings of analytical and numerical calculations, as interpreted by a TPBS concept by such impurity or nonlinearity induced modes, by plotting various TPBS parameters against the Landau coefficient and %impurity content. This new approach may lead to many interesting applications for device manufacture.
Keywords: Pinning Transition, Two-phonon Bound State, Ferroelectrics.
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Pinning is an important aspect in ferroelectric switching behavior. Pinning is ascribed to the presence of impurities in such systems that have been probed by various workers with DFT and other methods. Here, we use a micro level approach based on a detailed calculations of two-phonon bound state (TPBS) based on our discrete Hamiltonian. All the TPBS parameters (calculated through Fourier Grid Hamiltonian method) against impurities show a clear pinning transition in the system.
(J. Appl. Phys., Vol. 110 (2011) 024104)

Discrete Breathers in Nonlinear LiNbO3 type Ferroelectrics

Abstract:
Ferroelectric materials, such as lithium niobate, show interesting non-linear hysteresis behavior that can be explained by a dynamical system analysis by using a non-linear Klein-Gordon (K-G) equation previously constructed from the Hamiltonian with Landau-Ginzburg two-well potential. In the discrete case [Phys. Rev.-B 81 (2010) 064104], the intrinsic localized modes were shown  to exist above the linear modes. Nonlinearity and discreteness of domain structures in ferroelectrics slab domains arrayed in the x-direction lead to breather solutions under different values of controlling parameters, such as interaction between the domains and damping term mainly due to pinning effect. Different types of classical breather solution, namely Hamiltonian, dissipative and moving breather solutions are shown by numerical simulation with data on actual ferroelectric materials.

Keywords: Discrete Breathers, Ferroelectrics, Localization, Non-Linearity.

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ILM was already shown to be present in lithium niobate due to discreteness of the K-G lattice and nonlinearity in our previous PRB paper. Here, 3D pictures are shown for these symmetric discrete breathers in a non-integrable K-G system through spectral collocation method with good accuracy against different values of coupling and damping. An increase of coupling gives rise to bi- and tri-breathers.
(J. Appl. Phys., Vol. 109 (2011) 054105)

Importance of Damping in Nano Switching in LiNbO3 type Ferroelectrics

Abstract:
In a previous dynamic study of some ferroelectric materials showing memory switching behavior, a Hamiltonian was developed that gave rise to a non-linear Duffing oscillator equation involving Landau-Ginzburg free energy functional as a potential formulation (J. Appl. Phys. 100, 114106 (2006)). A high level of oscillations were observed in polarization waves against non-dimensional time that was quenched by increasing damping which is a decay constant relating to the loss of polarization due to damping during its motion in a ferroelectric material, such as lithium niobate. From the computer simulation of the damped oscillation curves, a critical time for switching, say, in a nanoswitch, was found that varies with the damping coefficient. This damping was also found to show an increasing behavior with the coercive field or amount of impurities in a quadratic manner in such ferroelectrics.
Keyword: Duffing Oscillator Equation, Ferroelectrics, Damping, Switching, Impurities.
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In a system of ferroelectrics, when the interaction or coupling between the domains tends to zero, then the spatial term vanishes, and NLKG equation gives rise to the nonlinear Duffing oscillator equation that is heavily damped. Importance of damping in lithium niobate ferroelectrics was shown against impurities which in turn influence the poling field. The critical time of switching is related to damping that shows a quadratic relation with poling field.
(Physica Scripta, Vol. 83 (2011) 015702)
 

Saturday, 9 June 2012

Solitons and Critical Breakup Fields in Lithium Niobate type Uniaxial Ferroelectrics

Ferroelectric materials, such as lithium niobate, show interesting non-linear hysteresis behavior that can be explained by a dynamical system analysis. By using variational principle, a non-linear Klein-Gordon (K-G) equation is derived for lithium niobate type of uniaxial ferroelectrics involving various types of energy, which was not considered previously to construct the Hamiltonian. This leads to soliton solutions under different conditions of soliton velocity. The critical value of the (dimensional) effective electric field has been estimated to be 54-58 kV/cm for lithium niobate depending on the impurity content in these type inhomogeneous ferroelectrics. Beyond this critical field, there is no existence of solitons. This critical field is related to a break-up mechanism of Landau-Ginzburg two-well potential to a single well, as the driving force is increased.

Keywords: Continuum Klein-Gordon, Critical Field, Impurity Variation, Soliton Motion.
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After our discrete Hamiltonian to describe spatio-temporal evolution of polarization, here we use a continuum case with several energy terms included in the Landau potential to make it a robust system. Here, also, we find the critical limit of solition motion, but with variation of the impuritie contents that influence the poling field in the system.
(Euro J. Phys.-B, 65 (2008) 525)

An Approach to Klein-Gordon Equation for a Dynamic Study in Ferroelectric Materials

The ferroelectric materials such as lithium niobate and lithium tantalate show a non-linear hysteresis behaviour, which may be explained by dynamical system analysis. The behaviour of these ferroelectrics are usually explained by domains and the domain wall movements. So, the spatial variation of the domain wall  was studied previously in order to see its effect on domain wall width in the context of Landau-Ginzburg functional. In the present work, both temporal and spatial variations of polarization are considered and by using Euler-Lagrange dynamical equation of motion, a Klein-Gordon equation is derived by taking the ferroelectrics as a Hamiltonian system. An interaction has been considered between the nearest neighbour domains, which are stacked sideways in a parallel array with uniform polarization. This interaction term is associated with the spatial term and when this interaction is assumed zero, the spatial term vanishes giving rise to a Duffing oscillator differential equation, which can be also studied by a dynamic system analysis.

Keywords: Klein-Gordon, Ferroelectrics, Spatial-Temporal Variation, Critical field for Soliton Motion.
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After spatial and temporal variation on domain wall and domain respectively, Klein-Gordon approach is adopted here to take cre of both spatial and temporal variation of polarization, eventually to find up to what critical field the soliton motion prevails in our system of ferroelectrics.
(J. Phys.: Condensed Matter, 18 (2006) 4093)

Dynamical Systems Analysis for Polarization in Ferroelectrics

The nonlinear hysteresis behavior of ferroelectric materials, such as lithium niobate ans lithium tantalate, may be explained by dynamic systems analysis. In a previous work, the polarization "domain wall width" was studied in terms of only spatial variation, and eventually critical values of polarization were determined to derive the stability zone in the context of Landau-Ginzburg free energy functional. In the present work, the temporal dynamics of the domains themselves are considered by taking the time variation through Euler-Lagrange dynamical equation of motion, which gives rise to a Duffing oscillator differential equation as a governing equation. From this nonlinear Duffing oscillator equation, three cases are studied theoretically: First, no electric field with and without any damping; secondly, taking the external field as static with damping; and finally, taking an oscillatory electric field with damping. After giving perturbation at the coercive field, the eigenvalues deduced through a Jacobian transformation on the perturbed matrix show interesting cases of stability and instability of polarization for different values of the electric field. The possibility of chaos at high oscillatory electric field is briefly explored merely as a limiting case in terms of the Lyapunov exponent spectrum in our particular ferroelectric system.

Keywords: Dynamical Systems, Euler-Lagrange Equation, Chaos, Lyapunov Exponents.
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After working with spatial perturbation (a rare case) in our previous paper, here we show the temporal perturbation on the ferroelectric domains themselves - showing chaos for the first time in ferroelecric systems as a limiting case.
(J. Appl. Phys., 100 (2006) 114106)

Perturbation Analysis & Memory in Ferroelectric Materials

Many ferroelectric materials like lithium niobate and lithium tantalate exhibit peculiar behavior in terms of showing large discrepancy between experimental and theoretical values of the coercive field by the use Landau-Ginzburg model. If perturbation is given at zero field, then there is also perturbation or fluctuation in polarization with respect to the nondimensional value of domain wall width. An eigenvalue problem is deduced through Jacobian transformation to show that there is a finite value of "memory", when  the perturbation in the electric field is lifted. The eigenvalue gives a characteristic value of polarization, which also gives rise to a zone of stability for polarization. This perturbation formalism  also allows the calculation of the limits of coercive field and, subsequently, the value of the domain-wall width can also be estimated, which shows both the lower and upper limits of theoretical values for both the above ferroelectric materials, deduced as the theoretical limits of the coercive fields. The theoretical framework is developed in this article.

(J. Appl. Physics, Vol. 95 (2004) 226)

Thursday, 7 June 2012

Multiple Time-Scale Analysis for Non-Linear Modes in Lithium Niobate Ferroelectrics

Abstract:

A model of a ferroelectric crystal in terms of a one-dimensional array of ferroelectric slab domains is treated theoretically for the dynamics of the ‘array of domains’.  Two approaches are considered.  In a first, the system is treated within a continuum limit in which the space and time evolution of the polarization of the crystal are described by a non-linear Klein-Gordon equation.  A multiple time-scale analysis (MTSA) is used to determine the linear and non-linear parts of the frequencies and amplitudes of the extended modes of oscillation of the array of domains.  An application is also made to study these modes in the presence of impurities in inhomogeneous ferroelectric materials such as lithium niobate.  In a second approach, the discrete equations for the coupling of neighboring ferroelectric slab domains are used to study intrinsic localized modes (ILM) of the ferroelectric crystal.  These are highly localized modes that arise from self-consistent interactions with the non-linearity of the system.

Keywords: Multiple-Time Scale Analysis (MTSA), Domains in Ferroelectrics, Linear & Nonlinear Modes.
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Intrinsic Localised Modes (ILM) was shown for the first time in ferroelectric materials with our discrete Hamiltonian. In this discrete model, ILM was formed also due to nonlinearity in the Klein-Gordon lattice.
(Phys. Rev. B, Vol. 81 (2010) 064104)

Femtosecond Response of Quantum Discrete Breathers in SRR based Metamaterials and the Role of Dielectric Permittivity

Abstract:

The quantum breathers (QB) state in terms of two-phonon bound state (TPBS) via detailed quantum calculations was already shown in ferroelectrics in a periodic boundary condition. In this work on metamaterials for application in antenna arrays as split-ring resonators (SRR), only the temporal variation of the number of quanta in a non-periodic boundary condition is detailed for a Klein-Gordon lattice. A generalized Hamiltonian containing dielectric permittivity is considered which was then quantized by bosonic operators to study the temporal evolution of quanta. Moreover, the time of redistribution of quanta that is proportional to QB’s lifetime in femtosecond shows significant variation with different quanta at different values of dielectric permittivity, which has implications in the applications in relevant devices.

Keywords: Dielectric Permittivity, Metamaterials, Quantum Breathers, Femtosecond Response.
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For the experimentalists, one has to theoretically study temporal evolution of the quanta and vary the relevant parameters eventually to optimize the results, and only then one could make the device applications, e.g. in making antenna arrays, modulation instability based gadgets, in making quantum metamaterials based superconductors, etc. These engineered materials can be used in the Quantum Computation. The temporal evolution of the quanta at the correct value of coupling and dielectric permittivity could enable the required quantum coding for applications. The proposed quantum metamaterials should allow the additional ways of controlling the ‘propagation’ of electromagnetic waves that are not possible by normal classical structures. Indeed, the coherent quantum dynamics of ‘qubits’ determines the THZ optical properties in the system.  Therefore, from the point of view of THz and other applications, the present study assumes particular importance, as this is also a new area of research.
(Quantum Phys Lett, In Press, 2012)

Wednesday, 6 June 2012

Quantum Breathers in Lithium Tantalate Ferroelectrics

Abstract:

Lithium tantalate is technologically one of the most important ferroelectric materials with a low poling field that has several applications in the field of photonics and memory switching devices. In a Hamiltonian system, such as dipolar system, the polarization behavior of such ferroelectrics can be well-modeled by Klein-Gordon (K-G) equation. Due to strong localization coupled with discreteness in a nonlinear K-G lattice, there is a formation of breathers and multi-breathers that manifest in the localization peaks across the domains in polarization-space-time plot. Due to the presence of nonlinearity and also impurities (as antisite tantalum defects) in the structure, dissipative effects are observed and hence dissipative breathers are studied here. To probe the quantum states related to discrete breathers, the same K-G lattice is quantized to give rise to quantum breathers (QBs) that are explained by a periodic boundary condition. The gap between the localized and delocalized phonon-band is a function of impurity content that is again related to the effect of pinning of domains due to antisite tantalum defects in the system, i.e. a point of easier switching within the limited amount of data on poling field, which is related to Landau coefficient (read, nonlinearity). Secondly, in a non-periodic boundary condition, the temporal evolution of quanta shows interesting behavior in terms of ‘critical’ time of redistribution of quanta that is proportional to QB’s lifetime in femtosecond having a possibility for THz applications.  Hence, the importance of both the methods for characterizing quantum breathers is shown in these perspectives.

Keywords: Ferroelectrics, Lithium Tantalate, Classical & Quantum Breathers.
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In the field of applied physics, one of the most investigated materials is ferroelectric, which has important applications as memory switching and in nonlinear optical communications, non-volatile memory devices, and many others. Lithium tantalate with a low poling field appears to be a promising candidate as a key photonic material for a variety of devices: such as optical parametric oscillators, nonlinear frequency converters, electro-optics, SAW devices and second-order nonlinear optical material, holography, etc. Many of such applications include important nano-devices.
(Applied NanoScience, In Press, 2012)

Sunday, 3 June 2012

About Myself......

I had my education and training in the field of research: first at Calcutta University and I.I.T. (Kanpur) on "Amorphous Semiconductors for Switching with Bismuth Nano Particles". I did my Ph.D. at Sheffield University (UK) on "Conductivity, Optical and ESR Spectroscopy of Transition Metal based Semiconductors". My Post-Doc exposure at Sussex University (Brighton, UK) was on "Solid State Battery Systems based on Suzuki Crystals doped with Cadmium". Then I moved to Montpellier (France) as a Scientist in CNRS working in close collaboration with various Labs in France, such as CNAM at Paris on "Auger Electron Spectroscopy for Surface Atom Detection", Small Angle Neutron Scattering at I.L.L. (Grenoble) for "Nucleation Studies on Basaltic Magmas", "Low Temperature & High Field Mossbauer Study" at CENG (Grenoble) and "Magetzation Study of Nano Magnetite Particles" at Louis Neel Lab at Grenoble (France). All these investigations were published in J. Mater. Sci., J. Non-crystalline Solids, J. Phys, D, etc. and were presented in several International Conferences. Notably, a part of the work on Amorphous Semiconductors was done in consultation with Nobel Leaureate Prof. Sir Neville Mott at Cavendish Lab in Cambridge (UK).
After working for about ten years with Multinationals on various materials problems in senior positions, I rejoined acdemia as Professor and then Principal of a 70 years old institute (GCECT) at Calcutta for another ten years. Presently, in associaton with West Bengal University of Technology (WBUT), Institute of Radiophysics & Electronics (Calcutta University) and National Institute of Technology, Durgapur, I have been engaged in the field of Nonlinear Optics in terms of "Dynamic System Analysis on Ferroelectrics (FE) and Metamaterials (MM)", starting with both "Continuum and Discrete Solitons based on our Hamiltonian", "Classical Discrete Breathers or ILMs", we have entered the new field of "Quantum Breathers in both FE and MM" -- particularly the latter in terms of both "Periodic & Non-periodic Boundary Conditions in Klein-Gordon Lattice" that has significant aplications  in "Quantum Computation" and Terrahertz Application. Moreover, very recently, I have embarked on "Fano Resonance and Rectification of Current Density through Ratchets" in MM. All these works were published in reputed International Journals, such as PRB, JAP, JPCM, EPJB etc. The total number of publications would be above 75 and more are coming soon.

Books Published:
1) Mathematical Physics for Engineers, New Age Sci. (Tunbridge Wells, Kent, UK, 2009)
2) Nano Materials, New Age Sci. (Tunbridge Wells, Kent, UK, 2010).